Chirality-Induced Propagation Velocity Asymmetry
Abstract
The spin-dependent propagation of electrons in helical nanowires is investigated. We show that the interplay of spin angular momentum and nanowire chirality, under spin-orbit interaction, lifts the symmetry between left and right propagating electrons, giving rise to a velocity asymmetry. The study is based on a microscopic tight-binding model that takes into account the spin-orbit interaction. The continuity equation for the spin-dependent probability density is derived, including the spin non-conserving terms, and quantum dynamics calculations are performed to obtain the electron propagating dynamics. The calculations are applied to the inorganic double-helix SnIP, a quasi-1D material that constitutes a semiconductor with a band gap of ~ 1.9 eV. The results, nevertheless, have general validity due to symmetry considerations. The relation of the propagation velocity asymmetry with the phenomena ascribed to the chiral-induced spin selectivity (CISS) effect is examined.
- Publication:
-
Nano Letters
- Pub Date:
- October 2021
- DOI:
- 10.1021/acs.nanolett.1c02636
- arXiv:
- arXiv:2109.03629
- Bibcode:
- 2021NanoL..21.8190H
- Keywords:
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- Condensed Matter - Materials Science
- E-Print:
- Nano Lett. 2021, 21, 8190-8196