Possible Topological Phase Transition in Fe-Vacancy-Ordered $\beta$-Fe$_{4+\delta}$Se$_{5}$ Nanowires
Abstract
We studied the electrical transport on $\beta$-Fe$_{4+\delta}$Se$_{5}$ single-crystal nanowires, exhibiting $\sqrt{5}\times\sqrt{5}$ Fe-vacancy order and mixed valence of Fe. We observed a first-order metal-insulator transition of the transition temperature at $\sim$28~K at zero magnetic field. The dielectric relaxation reveals that the transition is related to an energy gap expansion of $\sim$12~meV, involving the charge-orbital ordering. At nearly 28~K, colossal positive magnetoresistance emerges, resulting from the magnetic-field dependent shift of the transition temperature. Through the transition, the magnetotransport behavior transits from two-dimension-like to one-dimension-like conduction. The transition temperature demonstrates anisotropy with the $c$-axis as the preferred orientation in magnetic fields, suggesting the spin-orbital coupling. Our findings demonstrate the novel magnetoresistive transition intimating a topological transition in the Fe-vacancy-ordered $\beta$-Fe$_{4+\delta}$Se$_{5}$ nanowires. The results provide valuable information to better understand the orbital nature and the emergence of superconductivity in FeSe-based materials.
- Publication:
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arXiv e-prints
- Pub Date:
- April 2019
- DOI:
- 10.48550/arXiv.1904.13363
- arXiv:
- arXiv:1904.13363
- Bibcode:
- 2019arXiv190413363Y
- Keywords:
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- Condensed Matter - Superconductivity