A study of amorphous aerosol and ice particles in the Earth's atmosphere with polarization measurements
Abstract
Unlike crystals, amorphous solid particles do not have the long-range order (e.g., hydrogen-bond in ice). Organic substances tend to transition into amorphous phase (viscous secondary organic aerosols) upon drying of aqueous droplets (Mikhailov et al., 2017). There were studies suggesting that amorphous water/ice particles exist in the atmosphere as well (e.g., Nevzorov 2006; Murray et al., 2015). One of the key feature of these amorphous aerosol and cloud particles is the so-called "negative polarization" (polarization perpendicular to scattering plane) in near-backscatter angles. Here we will briefly introduce the optical properties of these particles and preliminary ob-servational studies using existing POLDER measurements. We will also briefly introduce a NASA/KASI CubeSat polarimeter concept that can provide most favorable viewing geometry for making these measurements.
References [1] Mikhailov, E., S. Vlasenko, S.T. Martin, T. Koop, and U. Pöschl, 2009: Amorphous and crystal-line aerosol particles interacting with water vapor: conceptual framework and experimental evi-dence for restructuring, phase transitions and kinetic limitations, Atmos. Chem. Phys., 9, 9491-952. [2] Murray, B.J. T.L. Malkin, C.G. Salzmann, 2015: The crystal structure of ice under mesospheri conditions. Journal of Atmospheric and Solar-Terrestrial Physics, 127, 78-82. https://doi.org/10.1016/j.jastp.2014.12.005. [3] Nevzorov, A.N., 2006, Some Properties of Metastable States of Water," Physics of Wave Phe-nomena 14(1), 45-57.- Publication:
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AGU Fall Meeting Abstracts
- Pub Date:
- December 2019
- Bibcode:
- 2019AGUFM.A13J2936H
- Keywords:
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- 0305 Aerosols and particles;
- ATMOSPHERIC COMPOSITION AND STRUCTURE;
- 0319 Cloud optics;
- ATMOSPHERIC COMPOSITION AND STRUCTURE;
- 0321 Cloud/radiation interaction;
- ATMOSPHERIC COMPOSITION AND STRUCTURE;
- 0360 Radiation: transmission and scattering;
- ATMOSPHERIC COMPOSITION AND STRUCTURE