Magnetically driven band shift and metal-insulator transition in spin-orbit-coupled S r3(Ir1-xR ux ) 2O7
Abstract
We report a combined infrared and angle-resolved photoemission study of the electronic response of S r3(Ir1-xR ux ) 2O7 (x =0 , 0.22, 0.34). The low-temperature optical conductivities of the three compounds exhibit the characteristic feature of the effective total angular momentum Jeff=1 /2 antiferromagnetic Mott state. As the temperature increases across the antiferromagnetic ordering temperature TN, the indirect gap gradually closes whereas the direct gap remains open. In the optical conductivity of S r3(Ir0.66Ru0.34 ) 2O7 which shows a thermally driven insulator-metal transition at TN, a Drude-like response from itinerant carriers is registered in the paramagnetic phase. We observe in angle-resolved photoemission data of S r3(Ir0.66Ru0.34 ) 2O7 that the valence band shifts continuously toward the Fermi energy with the weakening of the antiferromagnetic order and crosses the Fermi level in the paramagnetic phase. Our findings demonstrate that the temperature-induced metal-insulator transition of the S r3(Ir1-xR ux ) 2O7 system should be attributed to a magnetically driven band shift.
- Publication:
-
Physical Review B
- Pub Date:
- July 2018
- DOI:
- 10.1103/PhysRevB.98.035110
- Bibcode:
- 2018PhRvB..98c5110S