Trends in stratospheric HCl from the ACE satellite mission
Abstract
The Montreal Protocol has banned the production of long-lived chlorine-containing gases such as chlorofluorocarbons (CFCs) that deplete stratospheric ozone. These halogenated compounds ultimately form HCl in the upper atmosphere; the effectiveness of the Montreal Protocol can therefore be monitored by measuring stratospheric HCl. The Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) measures infrared solar occultation spectra of the Earth's atmosphere from which altitude profiles of HCl volume mixing ratios (VMRs) are determined. The upper stratospheric HCl VMR time series has a linear trend of -4.8 ± 0.2%/decade for 2004-2017, highlighting the continuing success of the Montreal Protocol.
- Publication:
-
Journal of Quantitative Spectroscopy and Radiative Transfer
- Pub Date:
- September 2018
- DOI:
- 10.1016/j.jqsrt.2018.05.027
- Bibcode:
- 2018JQSRT.217..126B
- Keywords:
-
- Atmospheric chemistry experiment;
- Fourier transform spectrometer;
- Satellite mission;
- Hydrochloric acid;
- Montreal Protocol;
- HCl trends