High-order harmonic generation in solid slabs beyond the single-active-electron approximation
Abstract
High-harmonic generation by a laser-driven solid slab is simulated using time-dependent density functional theory. Multiple harmonic plateaus up to very high harmonic orders are observed already at surprisingly low field strengths. The full all-electron harmonic spectra are, in general, very different from those of any individual Kohn-Sham orbital. Freezing the Kohn-Sham potential instead is found to be a good approximation for the laser intensities and harmonic orders considered. The origins of the plateau cutoffs are explained in terms of band gaps that can be reached by Kohn-Sham electrons and holes moving through the band structure.
- Publication:
-
Physical Review A
- Pub Date:
- November 2017
- DOI:
- 10.1103/PhysRevA.96.053418
- arXiv:
- arXiv:1710.04564
- Bibcode:
- 2017PhRvA..96e3418H
- Keywords:
-
- Physics - Atomic Physics;
- Condensed Matter - Other Condensed Matter;
- Quantum Physics
- E-Print:
- 9 pages, 8 figures, RevTeX 4.1