Estimated tetrachloroethylene (C2Cl4) emissions for 1992 2014 in China and a high resolution gridded emission in 2010

Estimated tetrachloroethylene (C2Cl4) emissions for 1992 2014 in China and a high resolution gridded emission in 2010 Pengju Bie1, Zhifang Li1, Jianxin Hu1,*1Collaborative Innovation Center for Regional Environmental Quality, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China *Corresponding author E-mail: jianxin@pku.edu.cnTel: 86-10-62756593 Fax: 86-10-62760755 Evaluating the contribution from tetrachloroethylene (C2Cl4, PCE) to stratospheric halogen loading requires the knowledge of the spatial and temporal variability of emissions, and thus the tropospheric degradation and removal. And the short atmospheric lifetime (90 days) leads to a large regional variability. This study estimated the emissions of China from 1992 to 2014, based on emission functions and aggregated information given reasonable uncertainties. Results show that the emissions increased from 5.3(3.8 7.0) Gg to 176.9(131.2 232.1) Gg with a moderate growth rate of 17.3%/yr during 1992 2014. More than 97.3% of emissions stemmed from solvents sector. Considering the GDP data availability and the comparable estimate to that of top-down method in 2010, we developed a gridded emission inventory on a 0.5°×0.5° latitude-longitude grid of this year. Due to the more advanced social-economic conditions and more intensive industrial establishment, greater PCE emissions were observed to originate from East China, especially for Jiangsu and Zhejiang provinces, and Beijing-Tianjin-Hebei region and Pearl River Delta (PRD) region.