Airborne Measurements of Scattering and Absorption Coefficients in the Planetary Boundary Layer above the Po Valley, Italy, during the PEGASOS Campaigns
Abstract
Aerosol particles influence the Earth's radiation budget by interacting with the incoming sunlight. The chemical composition and size of aerosol particles determine their potential to scatter and absorb radiation as well as their capability to take up water (Zieger et al., 2011). If particles are hygroscopic their optical properties will be altered at enhanced relative humidities (RH) due to the increase in size and change in index of refraction. It is known that RH but also the chemical composition of aerosols change with altitude (Morgan et al., 2010) which makes it very important to investigate optical properties at different heights. Within the Pan-European Gas-Aerosols-climate interaction Study (PEGASOS) a set of instruments was installed on a Zeppelin to investigate changes of light scattering and absorption in the planetary boundary layer. In order to obtain the scattering properties, Mie calculations were performed for size distributions recorded with SMPS (scanning mobility particle sizer) and WELAS (optical size spectrometer). The index of refraction and the hygroscopicity of the aerosol particles were measured with the white-light humidified optical particle spectrometer (WHOPS). These measurements further allowed studying the RH-dependence of the optical properties. Moreover, a seven wavelength portable aethalometer was employed to determine the light absorption properties of the aerosol. In this work we will present vertical profiles of scattering and absorption coefficients measured during Zeppelin flights of the PEGASOS campaigns in Italy in 2012. Additionally comparisons with ground based measurements from nephelometers and aethalometers, as well as remote sensing results will be shown. W.T. Morgan et al., Enhancement of the aerosol direct radiative effect by semi-volatile aerosol components: Airborne measurements in North-Western Europe, Atmospheric Chemistry and Physics 10(2010), pp. 8151-8171.P. Zieger et al., Comparison of ambient aerosol extinction coefficients obtained from in-situ, MAX-DOAS and LIDAR measurements at Cabauw, Atmospheric Chemistry and Physics 11(2011), pp. 2603-2624.
- Publication:
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AGU Fall Meeting Abstracts
- Pub Date:
- December 2014
- Bibcode:
- 2014AGUFM.A24B..07R
- Keywords:
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- 0305 Aerosols and particles;
- ATMOSPHERIC COMPOSITION AND STRUCTURE;
- 0345 Pollution: urban and regional;
- ATMOSPHERIC COMPOSITION AND STRUCTURE;
- 0360 Radiation: transmission and scattering;
- ATMOSPHERIC COMPOSITION AND STRUCTURE;
- 0365 Troposphere: composition and chemistry;
- ATMOSPHERIC COMPOSITION AND STRUCTURE