Analysis of Resonant Inelastic X-ray Scattering in Stripe-Ordered Nickelate
Abstract
We analyze theoretically the resonant inelastic x-ray scattering (RIXS) at the Ni K edge in the stripe-ordered state of La2-xSrxNiO4 at x=1/3. In the calculation of RIXS spectra, the stripe-ordered ground state is described within the Hartree--Fock approximation by using a realistic tight-binding model for Ni 3dγ and O 2px,y orbitals, and the electron correlations in the electronic excitation processes are taken into account within the random-phase approximation. The calculated RIXS spectrum shows a tail toward the low-energy region when the momentum transfer of photons equals the stripe vector \mbi{Q}, being consistent with a recent experimental result. The origin of this anomalous momentum dependence of RIXS spectra is discussed microscopically.
- Publication:
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Journal of the Physical Society of Japan
- Pub Date:
- February 2012
- DOI:
- 10.1143/JPSJ.81.024707
- arXiv:
- arXiv:1110.3141
- Bibcode:
- 2012JPSJ...81b4707N
- Keywords:
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- Condensed Matter - Strongly Correlated Electrons
- E-Print:
- 23 pages, 9 figures. Published version in J. Phys. Soc. Jpn