Dielectric response effects in time-resolved photoemission from metal surfaces
Abstract
We investigate dielectric response effects in attosecond time-resolved photoelectron (PE) spectra from metal surfaces. We model the response of the metal due to excitation of bulk and surface plasmons by the creation and propagation of the PE in terms of an effective potential that depends on the velocity of the PE. Using this dynamical image potential, we calculate IR-streaked XUV-photoemission spectra and compare them with spectra obtained with the corresponding static image potential. We find a significant relative temporal shift in photoemission from the conduction band for calculations with static and dynamical image potentials. We further analyze the dependence of this relative shift on the XUV frequency as well as on solid-state characteristics, such as the bulk plasmon frequency, the IR skin depth, and the PE transport in the solid.
Supported by the NSF and DOE.- Publication:
-
APS Division of Atomic, Molecular and Optical Physics Meeting Abstracts
- Pub Date:
- May 2011
- Bibcode:
- 2011APS..DMP.L1147Z