Subdiffusion and intermittent dynamic fluctuations in the aging regime of concentrated hard spheres
Abstract
We study the nonequilibrium aging dynamics in a system of quasihard spheres at large density by means of computer simulations. We find that, after a sudden quench to large density, the relaxation time initially increases exponentially with the age of the system. After a surprisingly large crossover time, the system enters the asymptotic aging regime characterized by a nearly linear increase in the relaxation time with age. In this aging regime, single-particle motion is strongly non-Fickian, with a mean-squared displacement increasing subdiffusively, associated with broad non-Gaussian tails in the distribution of particle displacements. We find that the system ages through temporally intermittent relaxation events, and a detailed finite-size analysis of these collective dynamic fluctuations reveals that these events are not spanning the entire system, but remain spatially localized.
- Publication:
-
Physical Review E
- Pub Date:
- September 2010
- DOI:
- 10.1103/PhysRevE.82.031503
- arXiv:
- arXiv:1006.4422
- Bibcode:
- 2010PhRvE..82c1503E
- Keywords:
-
- 64.70.qd;
- Thermodynamics and statistical mechanics;
- Condensed Matter - Statistical Mechanics
- E-Print:
- 11 pages