Crossover in magnetic properties of FeSi
Abstract
The magnetization of high quality iron monosilicide single crystals has been studied in a wide temperature and magnetic-field range. These data are analyzed by taking into account strong Hubbard correlations between eg and t2g states of Fe and the formation of spin polarons in the cubic FeSi matrix at low temperatures (T<100 K). These heavy particles are transformed into ferromagnetic microregions at Tc~15 K, which result in the appearance of the low-temperature anomalies in transport and thermodynamic properties of this compound. The suppression of the many-body resonance at EF occurs in FeSi at high temperatures, thus leading to the crossover in magnetic properties of FeSi. The transition to the temperature induced magnetic moments causes a dramatic increase of the magnetic susceptibility at temperatures T>100 K.
- Publication:
-
Physical Review B
- Pub Date:
- February 2002
- DOI:
- 10.1103/PhysRevB.65.064404
- Bibcode:
- 2002PhRvB..65f4404S
- Keywords:
-
- 75.50.Pp;
- 71.27.+a;
- Magnetic semiconductors;
- Strongly correlated electron systems;
- heavy fermions