Observation of saturation broadening of the coherent anti-stokes raman spectrum (cars) of acetylene in a pulsed molecular beam
Abstract
Reported is the first observation of saturation broadening in a high-resolution coherent Raman spectrum of the v2 Q-branch of acetylene. The measured saturation broadening of 1050 MHz is significantly greater than the calculated ac Stark broadening of less than 100 MHz.
- Publication:
-
Chemical Physics Letters
- Pub Date:
- June 1981
- DOI:
- 10.1016/0009-2614(81)80103-0
- Bibcode:
- 1981CPL....80..253D