Systematic study of rotational decoherence with a trapped-ion planar rotor

Quantum rotors promise unique advantages for quantum sensing, quantum simulation, and quantum information processing. At present, a variety of systems ranging from nanoparticles to single molecules and trapped ions have demonstrated detection and control of rotational motion in and near the quantum regime. For future applications of quantum rotors, understanding their dynamics in the presence of ambient environments and decoherence will be critical. While other model quantum systems such as the harmonic oscillator have seen extensive experimental study of their decoherence dynamics, such experiments remain an open task for the rigid rotor. We present measurements of fundamental scaling relationships for decoherence of a quantum planar rotor realized with two trapped ions, and find excellent agreement with recent theoretical work.