Elastocaloric effect of the heavy-fermion system YbPtBi
Abstract
YbPtBi is one of the heavy-fermion systems with largest Sommerfeld coefficient $\gamma$ and is thus classified as a `super'-heavy fermion material. In this work, we resolve the long-debated question about the hierarchy of relevant energy scales, such as crystal-electric field (CEF) levels, Kondo and magnetic ordering temperature, in YbPtBi. Through measurements of the a.c. elastocaloric effect and generic symmetry arguments, we identify an \textit{elastic level splitting} that is uniquely associated with the symmetry-allowed splitting of a quartet CEF level. This quartet, which we identify to be the first excited state at $\Delta/k_\text B\approx1.6\,\rm K$ above the doublet ground state at ambient pressure, is well below the Kondo temperature $T_\text K\approx10\,\rm K$. Thus, our analysis provides strong support for models that predict that the heavy electron mass is a result of an enhanced degeneracy of the CEF ground state, i.e., a quasi-sextet in YbPtBi. At the same time, our study shows the potential of the a.c. elastocaloric effect to control and quantify strain-induced changes of the CEF schemes, opening a different route to disentangle the CEF energy scales from other relevant energy scales in correlated quantum materials.
- Publication:
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arXiv e-prints
- Pub Date:
- March 2023
- DOI:
- 10.48550/arXiv.2303.08770
- arXiv:
- arXiv:2303.08770
- Bibcode:
- 2023arXiv230308770G
- Keywords:
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- Condensed Matter - Strongly Correlated Electrons
- E-Print:
- 7 pages, three figures + Supplemental information