Griffiths-like phase close to the Mott transition
Abstract
We explore the coexistence region in the vicinity of the Mott critical end point employing a compressible cell spin- 1 / 2 Ising-like model. We analyze the case for the spin-liquid candidate κ -(BEDT-TTF) 2Cu 2(CN) 3, where close to the Mott critical end point metallic puddles coexist with an insulating ferroelectric phase. Our results are fourfold: (i) a universal divergent-like behavior of the Grüneisen parameter upon crossing the first-order transition line; (ii) based on scaling arguments, we show that within the coexistence region, for any system close to the critical point, the relaxation-time is entropy-dependent; (iii) we propose the electric Grüneisen parameter Γ E, which quantifies the electrocaloric effect; and (iv) we identify the metallic/insulating coexistence region as an electronic Griffiths-like phase. Our findings suggest that Γ E governs the dielectric response close to the critical point and that an electronic Griffiths-like phase emerges in the coexistence region.
- Publication:
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Journal of Applied Physics
- Pub Date:
- December 2020
- DOI:
- arXiv:
- arXiv:2003.11866
- Bibcode:
- 2020JAP...128v5102M
- Keywords:
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- Condensed Matter - Strongly Correlated Electrons;
- Condensed Matter - Materials Science;
- Condensed Matter - Other Condensed Matter
- E-Print:
- 7 pages, 3 figures (suppl. material upon request). To appear in Journal of Applied Physics