Superconducting spin-valve effect in heterostructures with ferromagnetic Heusler alloy layers

We report a comparative analysis and theoretical description of the superconducting properties of two spin-valve-valve structures containing the Heusler alloy Co₂Cr_{1 -x}Fe_xAl_y as one of two ferromagnetic (F1 or F2) layers of the F1/F2/S structure, where S stands for the superconducting Pb layer. In our experiments, we used the Heusler alloy layer in two roles: as a weak ferromagnet on the place of the F2 layer and as a half-metal on the place of the F1 layer. In the first case, we obtained a large ordinary superconducting spin-valve effect Δ T_c assisted by the triplet superconducting spin-valve effect Δ T_c^trip . In the second case, we observed a giant magnitude of Δ T_c^trip reaching 0.5 K. An underlying theory based on the solution of the Usadel equations using Kupriyanov-Lukichev boundary conditions with arbitrary material parameters for all layers and arbitrary boundary parameters for all interfaces is presented in the Appendix. We find a good agreement between our experimental data and theoretical results.