Does a Growing Static Length Scale Control the Glass Transition?
Abstract
Several theories of the glass transition propose that the structural relaxation time τα is controlled by a growing static length scale ξ that is determined by the free energy landscape but not by the local dynamic rules governing its exploration. We argue, based on recent simulations using particle-radius-swap dynamics, that only a modest factor in the increase in τα on approach to the glass transition may stem from the growth of a static length, with a vastly larger contribution attributable, instead, to a slowdown of local dynamics. This reinforces arguments that we base on the observed strong coupling of particle diffusion and density fluctuations in real glasses.
- Publication:
-
Physical Review Letters
- Pub Date:
- November 2017
- DOI:
- 10.1103/PhysRevLett.119.195501
- arXiv:
- arXiv:1705.06588
- Bibcode:
- 2017PhRvL.119s5501W
- Keywords:
-
- Condensed Matter - Disordered Systems and Neural Networks
- E-Print:
- Phys. Rev. Lett. 119, 195501 (2017)