Seasonal, Spatial, and Long-term Variability of Fine Mineral Dust in the United States
Abstract
Characterizing the seasonal, spatial, and long-term variability of fine mineral dust (FD) is important to assess its environmental and climate impacts. FD concentrations (mineral particles with aerodynamic diameters less than 2.5 µm) were estimated using ambient, ground-based PM2.5 elemental chemistry data from over 160 remote and rural Interagency Monitoring of Protected Visual Environments (IMPROVE) sites from 2011 through 2015. FD concentrations were highest and contributed over 50% of PM2.5 mass at southwestern sites in spring and across the central and southeastern United States in summer (20-30% of PM2.5). The highest seasonal variability in FD occurred at sites in the Southeast during summer, likely associated with impacts from North African transport, which was also evidenced in the elemental ratios of calcium, iron, and aluminum. Long-term trend analyses (2000-2015) indicated widespread, regional increases in FD concentrations during spring in the West, especially in March in the Southwest. This increase was associated with an early onset of the spring dust season and correlated with the Pacific Decadal Oscillation and the El Niño Southern Oscillation. The Southeast and central United States also experienced increased FD concentrations during summer and fall, respectively. Contributions of FD to PM2.5 mass have increased in regions across the United States during all seasons, in part due to increased FD concentrations but also as a result of reductions in secondary aerosols (e.g., sulfates, nitrates, and organic carbon). Increased levels of FD have important implications for its environmental and climate impacts; mitigating these impacts will require identifying and characterizing source regions and underlying mechanisms for dust episodes.
- Publication:
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AGU Fall Meeting Abstracts
- Pub Date:
- December 2017
- Bibcode:
- 2017AGUFM.A22G..01H
- Keywords:
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- 0305 Aerosols and particles;
- ATMOSPHERIC COMPOSITION AND STRUCTURE;
- 3322 Land/atmosphere interactions;
- ATMOSPHERIC PROCESSES;
- 0414 Biogeochemical cycles;
- processes;
- and modeling;
- BIOGEOSCIENCES;
- 1622 Earth system modeling;
- GLOBAL CHANGE