Origin of uranium isotope variations in early solar nebula condensates
Abstract
High temperature condensates found in meteorites display uranium isotopic variations (235U/238U) that complicate dating of the formation of the Solar System and whose origin remains mysterious. It is possible that these variations are due to decay of the short-lived radionuclide 247Cm (t1/2=15.6 Myr) into 235U but they could also be due to uranium kinetic isotopic fractionation during condensation. We report uranium isotope measurements of meteoritic refractory inclusions that reveal excesses of 235U reaching ~+6 % relative to average solar system composition, which can only be due to decay of 247Cm. This allows us to constrain the 247Cm/235U ratio at Solar System formation to (7.0 +- 1.6) x 10-5. This value provides new clues on the universality of nucleosynthetic r-process of rapid neutron capture.
- Publication:
-
Science Advances
- Pub Date:
- March 2016
- DOI:
- 10.1126/sciadv.1501400
- arXiv:
- arXiv:1603.01780
- Bibcode:
- 2016SciA....2E1400T
- Keywords:
-
- Astrophysics - Solar and Stellar Astrophysics
- E-Print:
- 51 pages, 3 figures, 1 table, 22 supplementary figures, 8 supplementary tables