Invited Article: High resolution angle resolved photoemission with tabletop 11 eV laser
Abstract
We developed a table-top vacuum ultraviolet (VUV) laser with 113.778 nm wavelength (10.897 eV) and demonstrated its viability as a photon source for high resolution angle-resolved photoemission spectroscopy (ARPES). This sub-nanosecond pulsed VUV laser operates at a repetition rate of 10 MHz, provides a flux of 2 × 1012 photons/s, and enables photoemission with energy and momentum resolutions better than 2 meV and 0.012 Å-1, respectively. Space-charge induced energy shifts and spectral broadenings can be reduced below 2 meV. The setup reaches electron momenta up to 1.2 Å-1, granting full access to the first Brillouin zone of most materials. Control over the linear polarization, repetition rate, and photon flux of the VUV source facilitates ARPES investigations of a broad range of quantum materials, bridging the application gap between contemporary low energy laser-based ARPES and synchrotron-based ARPES. We describe the principles and operational characteristics of this source and showcase its performance for rare earth metal tritellurides, high temperature cuprate superconductors, and iron-based superconductors.
- Publication:
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Review of Scientific Instruments
- Pub Date:
- January 2016
- DOI:
- arXiv:
- arXiv:1509.01311
- Bibcode:
- 2016RScI...87a1301H
- Keywords:
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- Physics - Instrumentation and Detectors;
- Condensed Matter - Strongly Correlated Electrons
- E-Print:
- 12 pages, 10 figures