The performance of Yonsei CArbon Retrieval (YCAR) algorithm with improved aerosol information using GOSAT measurements over East Asia

The Greenhouse Gases Observing SATellite (GOSAT) is the first satellite dedicated to measure atmospheric CO2 concentrations from space that can able to improve our knowledge about carbon cycle. Several studies have performed to develop the CO2 retrieval algorithms using GOSAT measurements, but limitations in spatial coverage and uncertainties due to aerosols and thin cirrus clouds are still remained as a problem for monitoring CO2 concentration globally. In this study, we develop the Yonsei CArbon Retrieval (YCAR) algorithm based on optimal estimation method to retrieve the column-averaged dry-air mole fraction of carbon dioxide (XCO2) with optimized a priori CO2 profiles and aerosol models over East Asia. In previous studies, the aerosol optical properties (AOP) and the aerosol top height used to cause significant errors in retrieved XCO2 up to 2.5 ppm. Since this bias comes from a rough assumption of aerosol information in the forward model used in CO2 retrieval process, the YCAR algorithm improves the process to take into account AOPs as well as aerosol vertical distribution; total AOD and the fine mode fraction (FMF) are obtained from the ground-based measurements closely located, and other parameters are obtained from a priori information. Comparing to ground-based XCO2 measurements, the YCAR XCO2 product has a bias of 0.59±0.48 ppm and 2.16±0.87 ppm at Saga and Tsukuba sites, respectively, showing lower biases and higher correlations rather than the GOSAT standard products. These results reveal that considering better aerosol information can improve the accuracy of CO2 retrieval algorithm and provide more useful XCO2 information with reduced uncertainties.