Longitudinal magnetic excitation in KCuCl3 studied by Raman scattering under hydrostatic pressures

We measure Raman scattering in an interacting spin-dimer system KCuCl₃ under hydrostatic pressures up to 5 GPa mediated by He gas. In the pressure-induced quantum phase, we observe a one-magnon Raman peak, which originates from the longitudinal magnetic excitation and is observable through the second-order exchange interaction Raman process. We report the pressure dependence of the frequency, halfwidth and Raman intensity of this mode.