Neutron scattering and scaling behavior in URu2Zn20 and YbFe2Zn20
Abstract
The dynamic susceptibility χ″(ΔE) , measured by inelastic neutron-scattering measurements, shows a broad peak centered at Emax=15meV for the cubic actinide compound URu2Zn20 and 7 meV at zone center and at the (1/2, 1/2, 1/2) zone boundary for the rare-earth counterpart compound YbFe2Zn20 . For URu2Zn20 , the low-temperature susceptibility and magnetic specific-heat coefficient γ=Cmag/T take the values χ=0.011emu/mole and γ=190mJ/moleK2 at T=2K . These values are roughly three times smaller, and Emax is three times larger, than recently reported for the related compound UCo2Zn20 , so that χ and γ scale inversely with the characteristic energy for spin fluctuations, Tsf=Emax/kB . While χ(T) , Cmag(T) , and Emax of the 4f compound YbFe2Zn20 are very well described by the Kondo impurity model, we show that the model works poorly for URu2Zn20 and UCo2Zn20 , suggesting that the scaling behavior of the actinide compounds arises from spin fluctuations of itinerant 5f electrons.
- Publication:
-
Physical Review B
- Pub Date:
- November 2010
- DOI:
- arXiv:
- arXiv:1003.3484
- Bibcode:
- 2010PhRvB..82r4407W
- Keywords:
-
- 71.27.+a;
- 72.15.Qm;
- 75.20.Hr;
- Strongly correlated electron systems;
- heavy fermions;
- Scattering mechanisms and Kondo effect;
- Local moment in compounds and alloys;
- Kondo effect valence fluctuations heavy fermions;
- Condensed Matter - Strongly Correlated Electrons
- E-Print:
- 7 pages, 5 figures