Dynamics of a one-dimensional Holstein polaron with the Davydov ansätze
Abstract
Following the Dirac-Frenkel time-dependent variational principle, dynamics of a one-dimensional Holstein polaron is probed by employing the Davydov D2 ansatz with two sets of variational parameters, one for each constituting particle in the exciton-phonon system, and a simplified variant of the Davydov D1 ansatz, also known as the D∼ ansatz, with an additional set of phonon displacement parameters. A close examination of variational outputs from the two trial states reveals fine details of the polaron structure and intricacies of dynamic exciton-phonon interactions. Superradiance coherence sizes, speeds of exciton-induced phonon wave packets, linear optical absorption, and polaron energy compositions are also included in the study.
- Publication:
-
Physical Review B
- Pub Date:
- July 2010
- DOI:
- arXiv:
- arXiv:1001.3198
- Bibcode:
- 2010PhRvB..82a4305S
- Keywords:
-
- 63.20.kk;
- 03.65.Yz;
- 78.20.Bh;
- Phonon interactions with other quasiparticles;
- Decoherence;
- open systems;
- quantum statistical methods;
- Theory models and numerical simulation;
- Condensed Matter - Materials Science;
- Condensed Matter - Strongly Correlated Electrons
- E-Print:
- 14 pages and 11 figues