Particle Fluxes Over a Ponderosa Pine Plantation

Atmospheric aerosols can affect visibility, climate, and health. Particle fluxes were measured continuously over a 15 year-old ponderosa pine plantation in the foothills of the Sierra Nevada from mid July to the end of September in the year 2005. Air at this field site is affected by both biogenic emissions from the dense forests of the surrounding area and by urban pollution transported from the Sacramento valley. It is believed that fluxes of very reactive hydrocarbons from plants to the atmosphere have an impact on the production and growth of atmospheric particles at this site. Two condensation particle counters (CPCs) were located near the top of a 12 m measurement tower, several meters above the top of the tree canopy. Particle count data was collected at 10 Hz and particle fluxes were determined using the eddy covariance method. A set of diffusion screens was added to the inlet of one of the CPCs such that the lower particle size limit for detection was increased to a diameter of approximately 40 nm. The other CPC counted particles with minimum diameters of 3 nm. Particle concentrations showed a distinct diurnal pattern with minimum daily average concentrations of 2000 particles cm-3 occurring at dawn, and average daily maximum concentrations of 5700 particles cm-3 occurring at dusk. The evening increase of particle number corresponded to the arrival of polluted air from the Sacramento region. During the day, deposition of particles to the forest canopy (daytime average of 5.8x106 particles m-2 s-1 was generally observed. Concentrations and fluxes of particles under 40 nm could be examined by subtracting the data of one CPC from the other. On average, the fraction of particles under 40 nm increased from less than 20% at dawn to more than 50% at dusk; indicating that air coming from the Sacramento region was enriched in smaller, newly formed aerosol. Daily average deposition fluxes of particles under 40 nm were 1.0x107 particles m-2 s-1. Much of this flux was due to large deposition fluxes during the final three weeks of the experiment. Deposition of particles above 40 nm averaged 1.0x106 particles m-2 s-1. Deposition velocities for the particles under 40 nm were typically between 1 and 10 mm s-1. Particle deposition was correlated most strongly with temperature, and also showed some correlation with relative humidity, particle number concentration, and ozone.