We present FWHM = 5 to 8 Å optical spectra of nine previously unknown quasars (QSOs) drawn from the Calan/Tololo Survey. We have chosen this sample based on QSO redshift, z>3, and the presence of either candidate damped Lyalpha (DLA) or Lyman-limit (LL) systems in their spectra. The spectra show at least 9 DLA systems at redshifts 2.25<z<3.26, which are identified by the shape and strength of the H I-Lyalpha absorption line, by the presence of Lybeta and low-ionization metal lines at the same redshift, and - in most cases - by the observed Lyman-break. We thus provide the astronomical community with new interesting targets for high resolution spectroscopy on large telescopes. We describe all the spectra with emphasis on the most outstanding DLA and LL systems found. Based on observations made at the European Southern Observatory, La Silla, Chile, and at the Cerro Tololo Interamerican Observatory, Chile, which is operated by AURA, Inc.