Track formation in SiO2 quartz and the thermal-spike mechanism
Abstract
α-quartz has been irradiated with heavy ions: 19F, 32S, and 63Cu at an energy of about 1 MeV/amu in order to cover a range of electronic stopping powers dE/dx between 2.4 and 9 keV/nm and 58Ni, 86Kr, 128Te, 129Xe, 181Ta, and 208Pb between 1 and 5.8 MeV/amu for dE/dx>7 keV/nm. The extent of the induced damage is determined using Rutherford backscattering ion channeling with a 2-MeV 4He beam. The damage cross section A is obtained using a Poisson law Fd=1-exp(-Aφt), where φ is the flux and t the irradiation time. This damage cross section is linked to the effective radius Re through the relation A=πR2e, where Re is the radius of an equivalent cylinder of damage. Using high-resolution electron microscopy, cylinders of amorphous matter have been observed, whose radius corresponds to Re when the track is continuous (i.e., for A>=1.3×10-13 cm2; Re>=2 nm). A thermal-spike model is applied to calculate the radii of the observed tracks assuming that the observed amorphous cylinders correspond to a rapid quench of a molten liquid phase along the ion path. The model is applied only when the latent track is continuous and cylindrical. A good agreement is obtained taking into account that the initial spatial energy deposition on the electrons depends on the ion velocity.
- Publication:
-
Physical Review B
- Pub Date:
- May 1994
- DOI:
- Bibcode:
- 1994PhRvB..4912457M
- Keywords:
-
- 61.80.Jh;
- 05.70.-a;
- 44.10.+i;
- 72.15.Lh;
- Ion radiation effects;
- Thermodynamics;
- Heat conduction;
- Relaxation times and mean free paths