High resolution Raman spectroscopy of complexes and clusters in molecular beams
Abstract
The DOE-sponsored project in this laboratory has two facets. The first is the development of methods of nonlinear Raman spectroscopy for application in studies of sparse samples. The second is the application of such methods to structural and dynamical studies of species in supersonic molecular beams. The progress we have made in both of these areas is described in this paper. The report is divided into five remaining sections. The first pertains to theoretical and experimental developments in Fourier transform stimulated emission spectroscopy and Fourier transform hole-burning spectroscopy. The second deals with progress in the development of ionization-detected stimulated Raman spectroscopies (IDSRS). The third describes results from the application of IDSRS methods to studies of jet-cooled benzene clusters. The fourth describes IDSRS results from studies of hydrogen-bonded complexes containing phenols. The fifth relates to studies of carbazole-Ar(n) clusters.
- Publication:
-
Unknown
- Pub Date:
- 1991
- Bibcode:
- 1991hrrs.rept.....F
- Keywords:
-
- Benzene;
- Carbazoles;
- Emission Spectra;
- High Resolution;
- Hole Burning;
- Molecular Beams;
- Phenols;
- Raman Spectroscopy;
- Stimulated Emission;
- Flat Surfaces;
- Fourier Transformation;
- Nonlinearity;
- Nuclear and High-Energy Physics