Magnetic Field-Induced Insulator-Semimetal Transition in a Pyrochlore Nd2Ir2O7

We investigate magnetotransport properties in a single crystal of pyrochore-type Nd₂Ir₂O₇. The metallic conduction is observed on the antiferromagnetic domain walls of the all-in-all-out-type Ir 5 d moment ordered insulating bulk state that can be finely controlled by an external magnetic field along [111]. On the other hand, an applied field along [001] induces the bulk phase transition from insulator to semimetal as a consequence of the field-induced modification of the Nd 4 f and Ir 5 d moment configurations. A theoretical calculation consistently describing the experimentally observed features suggests a variety of exotic topological states as functions of electron correlation and Ir 5 d moment orders, which can be finely tuned by the choice of rare-earth ion and magnetic field, respectively.