Analytic continuation average spectrum method for quantum liquids
Abstract
We revisit the problem of determining the real-frequency density response in quantum fluids via analytical continuation of imaginary-time quantum Monte Carlo data. We demonstrate that the average spectrum method (ASM) is capable of revealing resolved modes in the dynamic structure factor of both ortho-deuterium and liquid para-hydrogen, in agreement with experiments and quantum mode-coupling theories, while the maximum entropy approach yields only a smooth unimodal spectrum. Outstanding issues are discussed. Our work provides the first application of the ASM method in realistic off-lattice systems.
- Publication:
-
Journal of Chemical Physics
- Pub Date:
- August 2009
- DOI:
- arXiv:
- arXiv:0905.4148
- Bibcode:
- 2009JChPh.131e4502R
- Keywords:
-
- 61.20.Ja;
- 61.25.Em;
- 65.20.Jk;
- Computer simulation of liquid structure;
- Molecular liquids;
- Studies of thermodynamic properties of specific liquids;
- Condensed Matter - Other Condensed Matter;
- Condensed Matter - Quantum Gases
- E-Print:
- 7 pages, 2 figures