Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe2
Abstract
Two-dimensional transition metal dichalcogenide semiconductors are intriguing hosts for quantum light sources due to their unique opto-electronic properties. Here we report that strain gradients induced by substrate patterning result in spatially and spectrally isolated quantum emitters in mono- and bi-layer WSe2. By correlating localized excitons with localized strain-variations, we show that the quantum emitter emission energy can be red-tuned up to a remarkable ~170 meV. We probe the fine-structure, magneto-optics, and second order coherence of a strained emitter. These results raise the prospect to strain-engineer quantum emitter properties and deterministically create arrays of quantum emitters in two-dimensional semiconductors.
- Publication:
-
Nano Letters
- Pub Date:
- November 2015
- DOI:
- 10.1021/acs.nanolett.5b03312
- arXiv:
- arXiv:1509.01085
- Bibcode:
- 2015NanoL..15.7567K
- Keywords:
-
- Condensed Matter - Mesoscale and Nanoscale Physics
- E-Print:
- 6 pages, 4 figures